If I'm correct, a DVD generally cannot have a single file that is larger than 2GB on it. You can put more than 2GB's worth of data on, but not as a single file. This wiki link has more info:
http://en.wikipedia.org/wiki/ISO_9660 The section called "The 2 GiB (or 4.2GB depending on implementation) file size limit" is of relevance here:
Quote:
Originally Posted by wikipedia.org
The 2 GiB (or 4.2GB depending on implementation) file size limit
Normally, a file on a ISO formatted disc cannot be larger than 2^31-1 in size, as the file's size is stored in a signed 32 bit value, for which 2^31-1 is the maximum.
It is, however, possible to circumvent this limitation by using the multi-extent (fragmentation) feature of ISO 9660 Level 3. With this, files larger than 2GB can be split up into multiple extents (sequential series of sectors), each not exceeding the 2GB limit.
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If you can change the settings of your CD burning software to Level 3 ISO, it should be able to handle individual files larger than 2GB.
Or, just make 2 tarballs which are less than 2GB each.
Hope this helps.
edit: mksisofs, which is probably what most burning software uses to write DVDs/CDs, is capable of writing Level 3 ISOs, so it seems it should be possible.