When you say "sync," what do you mean? Are you talking about the iTunes auto-sync that automatically makes the iPod reflect what's on the computer library, erasing what's on the iPod? I personally hate that feature, but is that what you're talking about?
If you're just talking about organization of music and drag-and-drop, I found Juk to be the best program for that. It took a really long time to build my library, but once it was up, it was simple to drag and drop songs to my MP3 player (SanDisk).
What kind of MP3 player do you have? What do you want to do, exactly?
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