You have to chroot into the installed system, make sure everything relevant is mounted (/ obviously, /boot, as well as bind-mounts for /proc /sys /dev /run ...)
Within the proper chroot environment, it should be a simple matter of updating the grub config and grub2-install /dev/sda, grub2-install /dev/sdb.
If that fails you will hopefully get an error message that will give some clue as to what else has to be done.
Quote:
The Centos 6 instructions say it must be installed separately on sda1 and sdb1.
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should be sda and sdb, you install bootloaders to disks, not individual partitions (even if the bootloader may use partitions in the end, but ...)
You should also show your partition table (parted /dev/disk unit s print free), /proc/mdstat (and perhaps mdadm --detail /dev/md*, mdadm --examine /dev/sd*), and tell us whether your system should boot UEFI or traditional BIOS style...?