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I would imagine you can't do it on a partition mounted read/write because it would be possible for data to be written/changed while it is making the image, and that wouldn't work so well. You could end up with all sorts of file corruption.
You can, however, rsync your important data onto another computer. Now this doesn't provide quite the same level of back, because you wouldn't just be able to restore the entire partition like you can with partimage, but at least you'd still have your data.
You aren't going to remount your root partition unless you can basically shut down all services. If this is a mission critical system something else you might want to look at is a Mirrored raid array. Linux provides good software raid tools so you don't have to purchase a raid adapter. It also has drivers for 3wares IDE raid adapters which I like a lot. They allow you to setup a hardware based raid array without breaking the bank.
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